I am excited to share that I will be joining the Department of Chemical Sciences at TIFR, Mumbai, as a tenure-track faculty member (Reader/Assistant Professor) in Spring 2025.
Thrilled to share our work published in
@NatureMaterials
. Here, we show how controlling exciton-phonon interactions drives exciton-polaron formation and subsequent carrier cooling in rigid DJ-type 2D perovskites at room temperature.
Congratulations Scholes Group and collaborators publishing today in
@NatureMaterials
: "Exciton polaron formation and hot-carrier relaxation in rigid Dion–Jacobson-type 2D perovskites." Well done Somnath, Greg et al.
Full paper here:
Element- and oxidation state-specific near-ambient pressure X-ray photoelectron spectroscopy reveals important roles of the chemical environment and solvation on underlying charge and spin transitions in molecular clusters.
@J_A_C_S
@osuchemistry
BREAKING NEWS
The Royal Swedish Academy of Sciences has decided to award the 2023
#NobelPrize
in Physics to Pierre Agostini, Ferenc Krausz and Anne L’Huillier “for experimental methods that generate attosecond pulses of light for the study of electron dynamics in matter.”
Observing and manipulating photoinduced band renormalization effects using a tabletop ultrafast setup and out-of-equilibrium formalism. A wonderful collaboration with Gregory D. Scholes, Ioannis Petrides,
@NarangLab
@SchoopLab
@PrincetonChem
Schoop.
Had a great time visiting the Pacific Northwest National Lab (
@PNNLab
) and learning about the research happening in the Physical Sciences Division at the Energy Sciences Center. Thanks to Dr. Niri Govind (
@NiriGovind
) for the seminar invitation and for being a wonderful host.
Recent progress of ultrafast XUV-RA spectroscopy to observe dynamics at surfaces by probing state-specific core-to-valence transitions.
@ACSPublications
This understanding underpins the advances in current and future generations of energy harvesting, information storage and processing, and quantum technologies.
Thanks to my mentors, collaborators, evaluators, family, and friends for their support!
Our group will develop and employ novel ultrafast spectroscopic techniques (Optical, and XUV/X-ray based) to reveal principles behind efficient transport and interconversion of energy between electron, spin, and nuclear degrees of freedom in functional materials.
@Mann_CharlieRay
@lindaunobel
@LChiappisi
Spectroscopist, trying to understand the solar energy conversion through X-ray spectroscopy. Hoping to improve the efficiency of next generation solar materials.
3. We demonstrate that exciton-phonon interaction can be controlled via targeted ligand design to manipulate the exciton-polaron population, carrier cooling, and phonon bottleneck formation.
2. Special displacement method shows that low-frequency phonon modes between 20-80 cm⁻¹ renormalize the excitonic transition energy. In this picture, the lattice reorganization energy (polaron stabilization energy) closely parallels solvent reorganization energies in solution.
1. Observation of the impulsive generation of low-frequency (20-80 cm⁻¹/0.6-2.4 THz) and highly polarizable phonons forming a molecular-like nuclear wavepacket, reorganizing and stabilizing the lattice via local distortion, establishes the formation of exciton-polaron.